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Formally Copper(III)−Alkylperoxo Complexes as Models of Possible Intermediates in Monooxygenase Enzymes

Reaction of [NBu(4)][LCu(II)OH] with excess ROOH (R = cumyl or tBu) yielded [NBu(4)][LCu(II)OOR], the reversible one-electron oxidation of which generated novel species with [CuOOR](2+) cores (formally Cu(III)OOR), identified by spectroscopy and theory for the case R = cumyl. This species reacts wit...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Neisen, Benjamin D., Gagnon, Nicole L., Dhar, Debanjan, Spaeth, Andrew D., Tolman, William B.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6132249/
https://ncbi.nlm.nih.gov/pubmed/28722408
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.7b05754
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