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Dehydrocoupling of phosphine–boranes using the [RhCp*Me(PMe(3))(CH(2)Cl(2))][BAr(F)(4)] precatalyst: stoichiometric and catalytic studies

We report a detailed, combined experimental and computational study on the fundamental B–H and P–H bond activation steps involved in the dehydrocoupling/dehydropolymerization of primary and secondary phosphine–boranes, H(3)B·PPhR′H (R = Ph, H), using [RhCp*(PMe(3))Me(ClCH(2)Cl)][BAr(F)(4)], to eithe...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Hooper, Thomas N., Weller, Andrew S., Beattie, Nicholas A., Macgregor, Stuart A.
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2016
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6003611/
https://ncbi.nlm.nih.gov/pubmed/29997783
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc04150c
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