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Water oxidation catalysed by iron complex of N,N′-dimethyl-2,11-diaza[3,3](2,6)pyridinophane. Spectroscopy of iron–oxo intermediates and density functional theory calculations
The macrocyclic [Fe(III)(L1)Cl(2)](+) (1, L1 = N,N′-dimethyl-2,11-diaza[3,3](2,6)pyridinophane) complex is an active catalyst for the oxidation of water to oxygen using [NH(4)](2)[Ce(IV)(NO(3))(6)] (CAN), NaIO(4), or Oxone as the oxidant. The mechanism of 1-catalysed water oxidation was examined by...
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| Publicat a: | Chem Sci |
|---|---|
| Autors principals: | , , , , , |
| Format: | Artigo |
| Idioma: | Inglês |
| Publicat: |
Royal Society of Chemistry
2015
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| Matèries: | |
| Accés en línia: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5950833/ https://ncbi.nlm.nih.gov/pubmed/29861914 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc01680k |
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