Configurational entropy measurements in extremely supercooled liquids that break the glass ceiling

Liquids relax extremely slowly on approaching the glass state. One explanation is that an entropy crisis, because of the rarefaction of available states, makes it increasingly arduous to reach equilibrium in that regime. Validating this scenario is challenging, because experiments offer limited reso...

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Bibliographic Details
Published in:Proc Natl Acad Sci U S A
Main Authors: Berthier, Ludovic, Charbonneau, Patrick, Coslovich, Daniele, Ninarello, Andrea, Ozawa, Misaki, Yaida, Sho
Format: Artigo
Language:Inglês
Published: National Academy of Sciences 2017
Subjects:
Physical Sciences
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC5664510/
https://ncbi.nlm.nih.gov/pubmed/29073056
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1706860114
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