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Remote stereoselective deconjugation of α,β-unsaturated esters by simple amidation reactions

The thermodynamically disfavored isomerization of α,β-unsaturated esters to deconjugated β,γ-unsaturated analogues occurs readily when coupled to an amidation. Within the framework of macrocyclic derivatives, it is shown that 15, 16, and 18 membered macrocycles react with tBuOK and anilines to gener...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Vishe, Mahesh, Hrdina, Radim, Poblador-Bahamonde, Amalia I., Besnard, Céline, Guénée, Laure, Bürgi, Thomas, Lacour, Jérôme
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5664367/
https://ncbi.nlm.nih.gov/pubmed/29142723
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc01118c
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