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A well-defined NHC–Ir(iii) catalyst for the silylation of aromatic C–H bonds: substrate survey and mechanistic insights

A well-defined NHC–Ir(iii) catalyst, [Ir(H)(2)(IPr)(py)(3)][BF(4)] (IPr = 1,3-bis-(2,6-diisopropylphenyl)imidazol-2-ylidene), that provides access to a wide range of aryl- and heteroaryl-silanes by intermolecular dehydrogenative C–H bond silylation has been prepared and fully characterized. The dire...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Rubio-Pérez, Laura, Iglesias, Manuel, Munárriz, Julen, Polo, Victor, Passarelli, Vincenzo, Pérez-Torrente, Jesús J., Oro, Luis A.
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5602144/
https://ncbi.nlm.nih.gov/pubmed/28959403
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc04899d
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