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Enantioselective CuH-Catalyzed Hydroacylation Employing Unsaturated Carboxylic Acids as Aldehyde Surrogates

The direct asymmetric copper hydride (CuH)-catalyzed coupling of α,β-unsaturated carboxylic acids to aryl alkenes is reported to access chiral α-aryl dialkyl ketones. A variety of substrate substitution patterns, sensitive functional groups and heterocycles are tolerated in this reaction, which sign...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Zhou, Yujing, Bandar, Jeffrey S., Buchwald, Stephen L.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5587210/
https://ncbi.nlm.nih.gov/pubmed/28565905
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.7b04937
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