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Ligand Field Strength Mediates Electron Delocalization in Octahedral [((H)L)(2)Fe(6)(L′)(m)](n)(+) Clusters

To assess the impact of terminal ligand binding on a variety of cluster properties (redox delocalization, ground-state stabilization, and breadth of redox state accessibility), we prepared three electron-transfer series based on the hexanuclear iron cluster [((H)L)(2)Fe(6)(L′)(m)](n+) in which the t...

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Publicado en:J Am Chem Soc
Autores principales: Sánchez, Raúl Hernández, Zheng, Shao-Liang, Betley, Theodore A.
Formato: Artigo
Lenguaje:Inglês
Publicado: 2015
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Acceso en línea:https://ncbi.nlm.nih.gov/pmc/articles/PMC5572642/
https://ncbi.nlm.nih.gov/pubmed/26231520
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b06453
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