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Base-Controlled Completely Selective Linear or Branched Rh(I)-Catalyzed C–H ortho-Alkylation of Azines without Preactivation

A [Rh(I)]/bisphosphine/base catalytic system for the ortho-selective C–H alkylation of azines by acrylates and acrylamides is reported. This catalytic system features an unprecedented complete linear or branched selectivity that is solely dependent on the catalytic base that is used. Complete branch...

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Bibliografiske detaljer
Udgivet i:Angew Chem Int Ed Engl
Main Authors: Tran, Gaël, Hesp, Kevin D., Mascitti, Vincent, Ellman, Jonathan A.
Format: Artigo
Sprog:Inglês
Udgivet: 2017
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5558092/
https://ncbi.nlm.nih.gov/pubmed/28429455
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201702409
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