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Palladium-Catalyzed Enantioselective Redox-Relay Heck Alkynylation of Alkenols to Access Propargylic Stereocenters

An enantioselective redox-relay Heck alkynylation of di- and trisubstituted alkenols to construct propargylic stereocenters is disclosed using a new pyridine oxazoline ligand. This strategy allows direct access to chiral β-alkynyl carbonyl compounds employing allylic alcohol substrates in contrast t...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Chen, Zhi-Min, Nervig, Christine S., DeLuca, Ryan J., Sigman, Matthew S.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5528850/
https://ncbi.nlm.nih.gov/pubmed/28467031
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201703089
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