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Mechanistic insights into the reductive dehydroxylation pathway for the biosynthesis of isoprenoids promoted by the IspH enzyme

Here, we report an integrated quantum mechanics/molecular mechanics (QM/MM) study of the bio-organometallic reaction pathway of the 2H(+)/2e(–) reduction of (E)-4-hydroxy-3-methylbut-2-enyl pyrophosphate (HMBPP) into the so called universal terpenoid precursors isopentenyl pyrophosphate (IPP) and di...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Abdel-Azeim, Safwat, Jedidi, Abdesslem, Eppinger, Jorg, Cavallo, Luigi
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5511988/
https://ncbi.nlm.nih.gov/pubmed/28757951
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc01693b
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