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In situ characterization of cofacial Co(IV) centers in Co(4)O(4) cubane: Modeling the high-valent active site in oxygen-evolving catalysts
The Co(4)O(4) cubane is a representative structural model of oxidic cobalt oxygen-evolving catalysts (Co-OECs). The Co-OECs are active when residing at two oxidation levels above an all-Co(III) resting state. This doubly oxidized Co(IV)(2) state may be captured in a Co(III)(2)(IV)(2) cubane. We demo...
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| Publicado no: | Proc Natl Acad Sci U S A |
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| Main Authors: | , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
National Academy of Sciences
2017
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5393202/ https://ncbi.nlm.nih.gov/pubmed/28348217 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1701816114 |
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