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Differences between the elimination of early and late transition metals: DFT mechanistic insights into the titanium-catalyzed synthesis of pyrroles from alkynes and diazenes

Early transition metals (TMs), such as titanium, generally resist undergoing reductive elimination to form C–X bonds due to their weak electronegativity. By analyzing the mechanism of the titanium-catalyzed synthesis of pyrroles from alkynes and diazenes, the present study revealed that titanium is...

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Foilsithe in:Chem Sci
Main Authors: Guo, Jiandong, Deng, Xi, Song, Chunyu, Lu, Yu, Qu, Shuanglin, Dang, Yanfeng, Wang, Zhi-Xiang
Formáid: Artigo
Teanga:Inglês
Foilsithe: Royal Society of Chemistry 2017
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Rochtain Ar Líne:https://ncbi.nlm.nih.gov/pmc/articles/PMC5369339/
https://ncbi.nlm.nih.gov/pubmed/28451348
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc04456e
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