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Continuous N-alkylation reactions of amino alcohols using γ-Al(2)O(3) and supercritical CO(2): unexpected formation of cyclic ureas and urethanes by reaction with CO(2)

The use of γ-Al(2)O(3) as a heterogeneous catalyst in scCO(2) has been successfully applied to the amination of alcohols for the synthesis of N-alkylated heterocycles. The optimal reaction conditions (temperature and substrate flow rate) were determined using an automated self-optimising reactor, re...

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Библиографические подробности
Опубликовано в: :Beilstein J Org Chem
Главные авторы: Streng, Emilia S, Lee, Darren S, George, Michael W, Poliakoff, Martyn
Формат: Artigo
Язык:Inglês
Опубликовано: Beilstein-Institut 2017
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Online-ссылка:https://ncbi.nlm.nih.gov/pmc/articles/PMC5331277/
https://ncbi.nlm.nih.gov/pubmed/28326142
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.3762/bjoc.13.36
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