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Total synthesis of (–)-spinosyn A

A convergent, highly stereoselective total synthesis of (–)-spinosyn A (1) is described. Key features of the synthesis include the transannular Diels–Alder reaction of macrocyclic pentaene 11 and the transannular Morita–Baylis–Hillman cyclization of 12 that generates tetracycle 26. The total synthes...

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Detalhes bibliográficos
Main Authors: Mergott, Dustin J., Frank, Scott A., Roush, William R.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2004
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC514415/
https://ncbi.nlm.nih.gov/pubmed/15173590
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0401247101
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