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Intermolecular Diels–Alder Cycloaddition for the Construction of Bicyclo[2.2.2]diazaoctane Structures: Formal Synthesis of Brevianamide B and Premalbrancheamide

A stereoselective intermolecular Diels–Alder cycloaddition of an intermediate pyrazinone with both achiral and chiral acrylate-derived dienophiles provides rapid access to the bicyclo[2.2.2]diazaoctane core shared among several prenylated indole alkaloids. The product derived from cycloaddition with...

Ausführliche Beschreibung

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Bibliographische Detailangaben
Veröffentlicht in:J Org Chem
Hauptverfasser: Robins, Jacob G., Kim, Kyu J., Chinn, Alex J., Woo, John S., Scheerer, Jonathan R.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2016
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC4993160/
https://ncbi.nlm.nih.gov/pubmed/26916112
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.joc.5b02744
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