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Palladium-Catalysis Enables Benzylation of α,α-Difluoroketone Enolates

S(N)1 and S(N)2-like alkylation reactions of ketone enolates with sp(3)-based electrophiles are essential transformations for generating α-substituted ketone products. However, alkylation reactions of weakly nucleophilic α,α-difluoroketone enolates with sp(3)-hybridized electrophiles remain nearly u...

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發表在:Angew Chem Int Ed Engl
Main Authors: Yang, Ming-Hsiu, Hunt, Jordan R., Sharifi, Niusha, Altman, Ryan A.
格式: Artigo
語言:Inglês
出版: 2016
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC4972046/
https://ncbi.nlm.nih.gov/pubmed/27312868
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201604149
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