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Mixed-Ligand Chiral Rhodium(II) Catalyst Enables the Enantioselective Total Synthesis of Piperarborenine B
A novel, mixed-ligand chiral rhodium(II) catalyst, Rh(2)(S-NTTL)(3)(dCPA), has enabled the first enantioselective total synthesis of the natural product piperarborenine B. A crystal structure of Rh(2)(S-NTTL)(3)(dCPA) reveals a “chiral crown” conformation with a bulky dicyclohexylphenyl acetate liga...
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| Publicado no: | Angew Chem Int Ed Engl |
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| Main Authors: | , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4900183/ https://ncbi.nlm.nih.gov/pubmed/26991451 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201600766 |
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