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Synthesis of Neurotrophic Seco-prezizaane Sesquiterpenes (1R,10S)-2-oxo-3,4-dehydroneomajucin, (2S)-hydroxy-3,4-dehydroneomajucin, and (−)-jiadifenin

An asymmetric approach to the synthesis of neurotrophic seco-prezizaane sesquiterpenes is described that is based on strategic application of a hydroxyl-directed metallacycle-mediated [2+2+2] annulation and an intramolecular radical cyclization cascade. Targets prepared are among the most potent mem...

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Bibliographic Details
Published in:J Am Chem Soc
Main Authors: Cheng, Xiayun, Micalizio, Glenn C.
Format: Artigo
Language:Inglês
Published: 2016
Subjects:
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC4879688/
https://ncbi.nlm.nih.gov/pubmed/26785051
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b12694
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