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Mechanistic Investigation of the Nickel-Catalyzed Suzuki Reaction of N,O-Acetals: Evidence for Boronic Acid Assisted Oxidative Addition and an Iminium Activation Pathway
The mechanism of a recently reported Suzuki coupling reaction of quinoline-derived allylic N,O-acetals has been studied using a combination of structural, stereochemical, and kinetic isotope effect experiments. The data indicate that C–O activation is facilitated by Lewis acid assistance from the bo...
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| 發表在: | J Am Chem Soc |
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| Main Authors: | , , |
| 格式: | Artigo |
| 語言: | Inglês |
| 出版: |
2012
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| 主題: | |
| 在線閱讀: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4807852/ https://ncbi.nlm.nih.gov/pubmed/23030789 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja3079362 |
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