Outer-Sphere Contributions to the Electronic Structure of Type Zero Copper Proteins

Bioinorganic canon states that active-site thiolate coordination promotes rapid electron transfer (ET) to and from type 1 copper proteins. In recent work, we have found that copper ET sites in proteins also can be constructed without thiolate ligation (called “type zero” sites). Here we report multi...

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Détails bibliographiques
Publié dans:J Am Chem Soc
Auteurs principaux: Lancaster, Kyle M., Zaballa, María-Eugenia, Sproules, Stephen, Sundararajan, Mahesh, DeBeer, Serena, Richards, John H., Vila, Alejandro J., Neese, Frank, Gray, Harry B.
Format: Artigo
Langue:Inglês
Publié: 2012
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Article
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC4794991/
https://ncbi.nlm.nih.gov/pubmed/22563915
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja302190r
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