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Asymmetric Synthesis of Highly Functionalized Tetrahydropyrans via a One-Pot Organocatalytic Michael/Henry/Ketalization Sequence

A diastereo- and enantioselective Michael/Henry/ketalization sequence to functionalized tetrahydropyrans is described. The multicomponent cascade reaction uses acetylacetone or β-keto esters, β-nitrostyrenes, and alkynyl aldehydes as substrates affording tetrahydropyrans with five contiguous stereoc...

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Detalhes bibliográficos
Publicado no:Org Lett
Main Authors: Hahn, Robert, Raabe, Gerhard, Enders, Dieter
Formato: Artigo
Idioma:Inglês
Publicado em: 2014
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4700516/
https://ncbi.nlm.nih.gov/pubmed/24971998
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol501236a
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