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Oxalates as Activating Groups for Alcohols in Visible Light Photoredox Catalysis: Formation of Quaternary Centers by Redox-Neutral Fragment Coupling

Alkyl oxalates are new bench-stable alcohol-activating groups for radical generation under visible light photoredox conditions. Using these precursors, the first net redox-neutral coupling of tertiary and secondary alcohols with electron-deficient alkenes is achieved.

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Nawrat, Christopher C., Jamison, Christopher R., Slutskyy, Yuriy, MacMillan, David W. C., Overman, Larry E.
Formato: Artigo
Idioma:Inglês
Publicado em: 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4632490/
https://ncbi.nlm.nih.gov/pubmed/26322524
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b07678
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