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Generation of the Methoxycarbonyl Radical by Visible-Light Photoredox Catalysis and Its Conjugate Addition with Electron-Deficient Olefins

Visible-light photoredox-catalyzed fragmentation of methyl N-phthalimidoyl oxalate allows the direct construction of a 1,4-dicarbonyl structural motif by a conjugate addition of the methoxycarbonyl radical to reactive Michael acceptors. The regioselectivity of the addition of this alkoxyacyl radical...

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Detalhes bibliográficos
Publicado no:Org Lett
Main Authors: Slutskyy, Yuriy, Overman, Larry E.
Formato: Artigo
Idioma:Inglês
Publicado em: 2016
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4892945/
https://ncbi.nlm.nih.gov/pubmed/27186995
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.6b00895
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