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Influence of Active Site Conformations on the Hydride Transfer step of the Thymidylate Synthase Reaction Mechanism

The hydride transfer from C6 of tetrahydrofolate to the reaction’s exocyclic methylene-dUMP intermediate is the rate limiting step in thymidylate synthase (TSase) catalysis. This step has been studied by means of QM/MM Molecular Dynamics simulations to generate the corresponding free energy surfaces...

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Bibliografske podrobnosti
izdano v:Phys Chem Chem Phys
Main Authors: Świderek, Katarzyna, Kohen, Amnon, Moliner, Vicent
Format: Artigo
Jezik:Inglês
Izdano: 2015
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC4605845/
https://ncbi.nlm.nih.gov/pubmed/25868526
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5cp01239b
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