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Consecutive radical S-adenosylmethionine methylations form the ethyl side chain in thienamycin biosynthesis

Despite their broad anti-infective utility, the biosynthesis of the paradigm carbapenem antibiotic, thienamycin, remains largely unknown. Apart from the first two steps shared with a simple carbapenem, the pathway sharply diverges to the more structurally complex members of this class of β-lactam an...

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Pubblicato in:Proc Natl Acad Sci U S A
Autori principali: Marous, Daniel R., Lloyd, Evan P., Buller, Andrew R., Moshos, Kristos A., Grove, Tyler L., Blaszczyk, Anthony J., Booker, Squire J., Townsend, Craig A.
Natura: Artigo
Lingua:Inglês
Pubblicazione: National Academy of Sciences 2015
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC4547291/
https://ncbi.nlm.nih.gov/pubmed/26240322
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1508615112
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