Llwytho...

Reaction Landscape of a Pentadentate N5-Ligated Mn(II) Complex with O(2)(•−) and H(2)O(2) Includes Conversion of a Peroxomanganese(III) Adduct to a Bis(μ-oxo)dimanganese(III,IV) Species

Herein we describe the chemical reactivity of the mononuclear [Mn(II)(N4py)(OTf)](OTf) (1) complex with hydrogen peroxide and superoxide. Treatment of 1 with one equivalent superoxide at −40 °C in MeCN formed the peroxomanganese(III) adduct, [Mn(III)(O(2))(N4py)](+) (2) in ~30% yield. Complex 2 deca...

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Wedi'i Gadw mewn:
Manylion Llyfryddiaeth
Cyhoeddwyd yn:Dalton Trans
Prif Awduron: Leto, Domenick F., Chattopadhyay, Swarup, Day, Victor W., Jackson, Timothy A.
Fformat: Artigo
Iaith:Inglês
Cyhoeddwyd: 2013
Pynciau:
Mynediad Ar-lein:https://ncbi.nlm.nih.gov/pmc/articles/PMC4498396/
https://ncbi.nlm.nih.gov/pubmed/23872704
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c3dt51277k
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