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Role of the Active Site Guanine in the glmS Ribozyme Self-Cleavage Mechanism: Quantum Mechanical/Molecular Mechanical Free Energy Simulations

[Image: see text] The glmS ribozyme catalyzes a self-cleavage reaction at the phosphodiester bond between residues A-1 and G1. This reaction is thought to occur by an acid–base mechanism involving the glucosamine-6-phosphate cofactor and G40 residue. Herein quantum mechanical/molecular mechanical fr...

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Publicat a:J Am Chem Soc
Autors principals: Zhang, Sixue, Ganguly, Abir, Goyal, Puja, Bingaman, Jamie L., Bevilacqua, Philip C., Hammes-Schiffer, Sharon
Format: Artigo
Idioma:Inglês
Publicat: American Chemical Society 2014
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC4308743/
https://ncbi.nlm.nih.gov/pubmed/25526516
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja510387y
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