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Enantioselective Synthesis of the Tricyclic Core of FR901483 Featuring a Rh-Catalyzed [2+2+2] Cycloaddition

[Image: see text] An efficient approach to the tricyclic framework of FR901483 is described. The sequence features a [3, 3]-sigmatropic rearrangement of a cyanate into an isocyanate, followed by its subsequent asymmetric rhodium-catalyzed [2+2+2] cycloaddition with a terminal alkyne for the synthesi...

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Detalhes bibliográficos
Publicado no:Synthesis (Stuttg)
Main Authors: Perreault, Stéphane, Rovis, Tomislav
Formato: Artigo
Idioma:Inglês
Publicado em: 2013
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4263289/
https://ncbi.nlm.nih.gov/pubmed/25506094
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1055/s-0032-1316786
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