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Transfer of Chirality in Rhodium-Catalyzed Intramolecular (5+2) Cycloaddition of 3-Acyloxy-1,4-enyne (ACE) and Alkyne: Enantioselective Synthesis of Bicyclo[5.3.0]decatrienes

[Image: see text] CHIRAL BICYCLIC: Bicyclo[5.3.0]decatrienes were prepared enantioselectively for the first time from readily available chiral 3-acyloxy-1,4-enynes (ACEs). The chirality of the allylic/propargylic esters in ACEs could be transferred with high efficiency to the bicyclic products in mo...

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Detalhes bibliográficos
Main Authors: Shu, Xing-zhong, Schienebeck, Casi M., Song, Wangze, Guzei, Ilia A., Tang, Weiping
Formato: Artigo
Idioma:Inglês
Publicado em: 2013
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3867534/
https://ncbi.nlm.nih.gov/pubmed/24150975
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201306919
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