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Enantioselective Direct α-Amination of Aldehydes via a Photoredox Mechanism: A Strategy for Asymmetric Amine Fragment Coupling

The direct, asymmetric α-amination of aldehydes has been accomplished via a combination of photoredox and organocatalysis. Photon-generated, nitrogen-centered radicals undergo enantioselective α-addition to catalytically formed chiral enamines to directly produce stable α-amino aldehyde adducts bear...

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Bibliographische Detailangaben
Hauptverfasser: Cecere, Giuseppe, Koenig, Christian M., Alleva, Jennifer L., MacMillan, David W. C.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2013
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC3786402/
https://ncbi.nlm.nih.gov/pubmed/23869694
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja406181e
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