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Asymmetric NHC-Catalyzed Addition of Enals to Nitroalkenes: Controlling Stereochemistry Via the Homoenolate Reactivity Pathway To Access δ-Lactams

An asymmetric intermolecular reaction between enals and nitroalkenes to yield δ-nitroesters has been developed, catalyzed by a novel chiral N-heterocyclic carbene. Key to this work was the development of a catalyst that favors the δ-nitroester pathway over the established Stetter pathway. The reacti...

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Bibliografiset tiedot
Päätekijät: White, Nicholas A., DiRocco, Daniel A., Rovis, Tomislav
Aineistotyyppi: Artigo
Kieli:Inglês
Julkaistu: 2013
Aiheet:
Linkit:https://ncbi.nlm.nih.gov/pmc/articles/PMC3723348/
https://ncbi.nlm.nih.gov/pubmed/23713683
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja403847e
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