NRVS and EPR Spectroscopy of (57)Fe-enriched [FeFe] Hydrogenase Indicate Stepwise Assembly of the H-cluster()

The [FeFe] hydrogenase from Clostridium pasteurianum (CpI) harbors four Fe–S clusters that facilitate electron transfer to the H-cluster, a ligand-coordinated six-iron prosthetic group that catalyzes the redox interconversion of protons and H(2). Here, we have used (57)Fe nuclear resonance vibration...

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Hauptverfasser: Kuchenreuther, Jon M., Guo, Yisong, Wang, Hongxin, Myers, William K., George, Simon J., Boyke, Christine A., Yoda, Yoshitaka, Alp, E. Ercan, Zhao, Jiyong, Britt, R. David, Swartz, James R., Cramer, Stephen P.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2013
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Article
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC3644562/
https://ncbi.nlm.nih.gov/pubmed/23249091
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/bi301336r
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