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Presence or absence of a novel charge-transfer complex in the base-catalyzed hydrolysis of N-ethylbenzamide or ethyl benzoate

Reaction paths of base-catalyzed hydrolyses of isoelectronic substrates, Ph–C(=O)–X–Et [X = O (ethyl benzoate) and X = NH (N-ethylbenzamide)], were traced by DFT calculations. To simulate bond interchanges accompanied by proton transfers, a cluster model of Ph–C(=O)–X–Et + OH(−)(H(2)O)(16) was emplo...

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Detalhes bibliográficos
Main Authors: Yamabe, Shinichi, Guan, Wei, Sakaki, Shigeyoshi
Formato: Artigo
Idioma:Inglês
Publicado em: Beilstein-Institut 2013
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3566851/
https://ncbi.nlm.nih.gov/pubmed/23400273
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.3762/bjoc.9.22
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