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Catalytic Enantioselective O–Nitrosocarbonyl Aldol Reaction of β–Dicarbonyl Compounds

The first example of Cu–catalyzed asymmetric O–nitrosocarbonyl aldol reaction is described. This novel protocol allows convenient access to highly enantioenriched α–hydroxy–β–ketoesters including the antibacterial natural product kjellmanianone (up to 99% ee). MnO(2) was introduced as a mild efficie...

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Hlavní autoři: Baidya, Mahiuddin, Griffin, Kimberly A., Yamamoto, Hisashi
Médium: Artigo
Jazyk:Inglês
Vydáno: 2012
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC3515642/
https://ncbi.nlm.nih.gov/pubmed/23106266
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja309311z
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