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Catalytic Enantioselective O–Nitrosocarbonyl Aldol Reaction of β–Dicarbonyl Compounds

The first example of Cu–catalyzed asymmetric O–nitrosocarbonyl aldol reaction is described. This novel protocol allows convenient access to highly enantioenriched α–hydroxy–β–ketoesters including the antibacterial natural product kjellmanianone (up to 99% ee). MnO(2) was introduced as a mild efficie...

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Détails bibliographiques
Auteurs principaux: Baidya, Mahiuddin, Griffin, Kimberly A., Yamamoto, Hisashi
Format: Artigo
Langue:Inglês
Publié: 2012
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC3515642/
https://ncbi.nlm.nih.gov/pubmed/23106266
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja309311z
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