Formation of a long-lived electron-transfer state in mesoporous silica-alumina composites enhances photocatalytic oxygenation reactivity

A simple donor-acceptor linked dyad, 9-mesityl-10-methylacridinium ion (Acr(+)-Mes) was incorporated into nanosized mesoporous silica-alumina to form a composite, which in acetonitrile is highly dispersed. In this medium, upon visible light irradiation, the formation of an extremely long-lived elect...

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Bibliographic Details
Main Authors: Fukuzumi, Shunichi, Doi, Kaoru, Itoh, Akinori, Suenobu, Tomoyoshi, Ohkubo, Kei, Yamada, Yusuke, Karlin, Kenneth D.
Format: Artigo
Language:Inglês
Published: National Academy of Sciences 2012
Subjects:
Chemical Approaches to Artificial Photosynthesis: Solar Fuels Special Feature
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC3465401/
https://ncbi.nlm.nih.gov/pubmed/22543164
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1119994109
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