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Epoxidation of olefins by cytochrome P-450 model compounds: mechanism of oxygen atom transfer.

The mechanism of the Mn(III) porphyrin-catalyzed epoxidation of olefins by lithium hypochlorite is examined. The active oxidant is thought to be a high-valent manganese-oxo complex. It is shown that a relatively stable intermediate is reversibly formed upon interaction of the olefin and the oxo comp...

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Bibliografiske detaljer
Udgivet i:Proc Natl Acad Sci U S A
Main Authors: Collman, J P, Brauman, J I, Meunier, B, Raybuck, S A, Kodadek, T
Format: Artigo
Sprog:Inglês
Udgivet: National Academy of Sciences 1984
Fag:
Online adgang:https://ncbi.nlm.nih.govhttps://pmc.ncbi.nlm.nih.gov/articles/PMC345259/
https://ncbi.nlm.nih.govhttps://pubmed.ncbi.nlm.nih.gov/6587349/
https://ncbi.nlm.nih.govhttps://doi.org/10.1073/pnas.81.10.3245
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