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Total Synthesis of (±)-Hirsutine: Application of Phosphine-Catalyzed Imine–Allene [4 + 2] Annulation

[Image: see text] The total synthesis of the indole alkaloid hirsutine has been achieved, with a key step being the application of our phosphine-catalyzed [4 + 2] annulation of an imine with ethyl α-methylallenoate. From commercially available indole-2-carboxaldehyde, the target was synthesized in 1...

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Détails bibliographiques
Auteurs principaux: Villa, Reymundo A., Xu, Qihai, Kwon, Ohyun
Format: Artigo
Langue:Inglês
Publié: 2012
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC3439149/
https://ncbi.nlm.nih.gov/pubmed/22920858
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol302077n
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