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EPR/ENDOR, Mössbauer, and Quantum Chemical Investigation of Di-iron Complexes Mimicking the Active Oxidized State of [FeFe] Hydrogenase

Understanding the catalytic process of the heterolytic splitting and formation of molecular hydrogen is one of the key topics for the development of a future hydrogen economy. With an interest in elucidating the enzymatic mechanism of the [Fe(2)(S(2)C(2)H(4)NH)(CN)(2)(CO)(2)(µ-CO)] active center uni...

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Detalhes bibliográficos
Main Authors: Silakov, Alexey, Olsen, Matthew T., Sproules, Stephen, Reijerse, Eduard J., Rauchfuss, Thomas B., Lubitz, Wolfgang
Formato: Artigo
Idioma:Inglês
Publicado em: 2012
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3420818/
https://ncbi.nlm.nih.gov/pubmed/22800196
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ic3013766
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