Spectroscopic and Crystallographic Characterization of ‘Alternative Resting’ and ‘Resting Oxidized’ Enzyme Forms of Bilirubin Oxidase: Implications for Activity and Electrochemical Behavior of Multicopper Oxidases

While there is broad agreement on the catalytic mechanism of Multicopper Oxidases (MCOs), the geometric and electronic structures of the resting trinuclear Cu cluster have been variable, and their relevance to catalysis debated. Here, we present a spectroscopic characterization, complimented by crys...

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Autores principales: Kjaergaard, Christian H., Durand, Fabien, Tasca, Federico, Qayyum, Munzarin F., Kaufmann, Brice, Gounel, Sébastien, Suraniti, Emmanuel, Hodgson, Keith O., Hedman, Britt, Mano, Nicolas, Solomon, Edward I.
Formato: Artigo
Lenguaje:Inglês
Publicado: 2012
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Article
Acceso en línea:https://ncbi.nlm.nih.gov/pmc/articles/PMC3339634/
https://ncbi.nlm.nih.gov/pubmed/22413777
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja211872j
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