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First total synthesis of (+)-Vedelianin, a potent antiproliferative agent

The total synthesis of (+)-vedelianin has been accomplished in 18 steps from vanillin. Preparation of a key intermediate in nonracemic form through a Shi epoxidation has allowed determination of the absolute stereochemistry of the natural product as the (2S, 3R, 4aR, 9aR)-isomer.

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Detalhes bibliográficos
Main Authors: Topczewski, Joseph J., Wiemer, David F.
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3204860/
https://ncbi.nlm.nih.gov/pubmed/22053119
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.tetlet.2011.01.137
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