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Incorporation of fluorotyrosines into ribonucleotide reductase using an evolved, polyspecific aminoacyl-tRNA synthetase
Tyrosyl radicals (Y•s) are prevalent in biological catalysis and are formed under physiological conditions by the coupled loss of both a proton and an electron. Fluorotyrosines (F(n)Ys, n=1–4) are promising tools for studying the mechanism of Y• formation and reactivity, as their pK(a)s and peak pot...
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| Main Authors: | , , , |
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| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2011
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3188361/ https://ncbi.nlm.nih.gov/pubmed/21913683 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja207719f |
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