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Spectral Diffusion at the Water/Lipid Interface Revealed by Two-Dimensional Fourth-Order Optical Spectroscopy: A Classical Simulation Study

Using a classical simulation protocol for nonlinear optical signals, we predict the two-dimensional (2D) spectra of water near a monolayer of [1,2-dimytristoyl-sn-glycero-3-phosphatidylcholine] (DMPC) generated by three infrared and one visible probe pulses. Sum frequency generation 1D spectra show...

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Detalhes bibliográficos
Main Authors: Nagata, Yuki, Mukamel, Shaul
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3101253/
https://ncbi.nlm.nih.gov/pubmed/21329386
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja110748s
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