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Role of the Azadithiolate Cofactor in Models for the [FeFe]-Hydrogenase: Novel Structures and Catalytic Implications

The report summarizes studies on the redox behavior of synthetic models for the [FeFe]-hydrogenases, consisting of diiron dithiolato carbonyl complexes bearing the amine cofactor and its N-benzyl derivative. Of specific interest are the causes of the low reactivity of oxidized models toward H(2), wh...

Ausführliche Beschreibung

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Bibliographische Detailangaben
Hauptverfasser: Olsen, Matthew T., Rauchfuss, Thomas B., Wilson, Scott R.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2010
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC3010399/
https://ncbi.nlm.nih.gov/pubmed/21114298
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja103998v
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