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Manganese Catalysts for C–H activation: An Experimental/Theoretical Study Identifies the Stereoelectronic Factor that Controls the Switch between Hydroxylation and Desaturation Pathways

We describe competitive C–H activation chemistry of two types, desaturation and hydroxylation, using synthetic manganese catalysts with several substrates. 9,10-dihydrophenanthrene (DHP) gives the highest desaturation activity, the final products being phenanthrene (P1) and phenanthrene-9,10-oxide (...

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Hlavní autoři: Hull, Jonathan F., Balcells, David, Sauer, Effiette L. O., Raynaud, Christophe, Brudvig, Gary W., Crabtree, Robert H., Eisenstein, Odile
Médium: Artigo
Jazyk:Inglês
Vydáno: 2010
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC2903729/
https://ncbi.nlm.nih.gov/pubmed/20481432
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja908744w
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