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Kinetic and Spectroscopic Studies of N694C Lipoxygenase: A Probe of the Substrate Activation Mechanism of a Non-Heme Ferric Enzyme

Lipoxygenases (LOs) comprise a class of substrate activating mononuclear non-heme iron enzymes which catalyze the hydroperoxidation of unsaturated fatty acids. A commonly proposed mechanism for LO catalysis involves H-atom abstraction by an Fe(III)-OH(-) site, best described as a proton coupled elec...

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Detalhes bibliográficos
Main Authors: Neidig, Michael L., Wecksler, Aaron T., Schenk, Gerhard, Holman, Theodore R., Solomon, Edward I.
Formato: Artigo
Idioma:Inglês
Publicado em: 2007
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2896304/
https://ncbi.nlm.nih.gov/pubmed/17523638
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja068503d
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