Probing static disorder in Arrhenius kinetics by single-molecule force spectroscopy

The widely used Arrhenius equation describes the kinetics of simple two-state reactions, with the implicit assumption of a single transition state with a well-defined activation energy barrier ΔE, as the rate-limiting step. However, it has become increasingly clear that the saddle point of the free-...

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Main Authors: Kuo, Tzu-Ling, Garcia-Manyes, Sergi, Li, Jingyuan, Barel, Itay, Lu, Hui, Berne, Bruce J., Urbakh, Michael, Klafter, Joseph, Fernández, Julio M.
Format: Artigo
Sprog:Inglês
Udgivet: National Academy of Sciences 2010
Fag:
Biological Sciences
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC2895103/
https://ncbi.nlm.nih.gov/pubmed/20534507
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1006517107
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