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Analysis of Kinetic Isotope Effects for Proton-Coupled Electron Transfer Reactions

A series of rate constant expressions for nonadiabatic proton-coupled electron transfer (PCET) reactions are analyzed and compared. The approximations underlying each expression are enumerated, and the regimes of validity for each expression are illustrated by calculations on model systems. In addit...

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Bibliografski detalji
Glavni autori: Edwards, Sarah, Soudackov, Alexander V., Hammes-Schiffer, Sharon
Format: Artigo
Jezik:Inglês
Izdano: 2009
Teme:
Online pristup:https://ncbi.nlm.nih.gov/pmc/articles/PMC2880663/
https://ncbi.nlm.nih.gov/pubmed/19182970
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jp809122y
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