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Driving force dependence of rates for nonadiabatic proton and proton-coupled electron transfer: Conditions for inverted region behavior

The driving force dependence of the rate constants for nonadiabatic electron transfer (ET), proton transfer (PT), and proton-coupled electron transfer (PCET) reactions are examined. Inverted region behavior, where the rate constant decreases as the reaction becomes more exoergic (i.e., as ΔG(0) beco...

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Autors principals: Edwards, Sarah, Soudackov, Alexander V., Hammes-Schiffer, Sharon
Format: Artigo
Idioma:Inglês
Publicat: 2009
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2783471/
https://ncbi.nlm.nih.gov/pubmed/19795899
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jp907808t
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